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Supramolecular polymers built from stimuli‐responsive host‐guest interactions represent an attractive way of tailoring smart materials. Herein, we exploit the chaotropic effect of polyoxometalates and related host‐guest properties to design unconventional polymer systems with reversible redox and thermo‐responsive sol‐gel transition. These supramolecular networks result from the association of cyclodextrin‐based...
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