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The persistent efforts to reveal the formation and evolution mechanisms of solid electrolyte interphase (SEI) are of fundamental significance for the rational regulation. In this work, through combined theoretical and experimental model investigations, we elucidate that the electric double layer (EDL) chemistry at the electrode/electrolyte interface beyond the thermodynamic stability of electrolyte...
Auf reaktiven Metallelektroden bildet sich vor der Festelektrolyt‐Interphase (SEI) eine elektrische Doppelschicht. In ihrem Forschungsartikel auf S. 4261 identifizieren Jia‐Qi Huang und Mitarbeiter die kritische Rolle der Chemie und Struktur der elektrischen Doppelschicht bei der Steuerung der Konkurrenzreaktionen während der SEI‐Bildung. Die Ergebnisse liefern Anhaltspunkte für ein gezieltes Grenzflächendesign,...
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