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Self‐assembly in a droplet: A supramolecular system that governs self‐assembly events over hierarchies from the nano‐ to the micrometer range has been developed by combining a bottom‐up strategy based on molecular programming with top‐down droplet microscience. Discrete 1D tubular structures were created by exploiting the compartment effect of the droplet, induced during dynamic shrinking under non‐equilibrium...
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