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A computational kinetic study was completed to elucidate the mechanism by which tetradecane is converted to hydrogen in an autothermal reforming process. A reaction mechanism was developed to capture the major autothermal reforming reactions, which was then validated using experimental data. A sensitivity study was performed to identify the reaction classes most influencing product formation. The...
This paper analyzes the mechanism of deactivation and methods of regeneration of a PtMoRe water gas shift catalyst supported on a stabilized zirconia. Although this catalyst initially possesses high activity below 250 °C, a decrease in CO conversion ranging from 10 to 50% was observed over a period of 60 h. To determine the mechanism responsible for the decay, a series of activity tests and high resolution...
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