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Eine promiskuitive aliphatische Halogenase, …… AmbO5, wurde in Biogenesestudien der Ambiguin‐Alkaloide entdeckt. X. Liu et al. zeigen in ihrer Zuschrift auf S. 5874 ff., dass AmbO5 sieben strukturell verschiedene Ambiguin‐, Fischerindol‐ und Hapalindol‐Alkaloide durch späte C‐H‐Funktionalisierung chlorieren kann. Die Charakterisierung eines C‐terminalen Sequenzmotivs in AmbO5, das für Substrattoleranz...
The elucidation of enigmatic enzymatic chlorination timing in ambiguine indole alkaloid biogenesis led to the discovery and characterization of AmbO5 protein as a promiscuous non‐heme iron aliphatic halogenase. AmbO5 was shown capable of selectively modifying seven structurally distinct ambiguine, fischerindole and hapalindole alkaloids with chlorine via late‐stage aliphatic C−H group functionalization...
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