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The ability of n‐type polymer thermoelectric materials to tolerate high doping loading limits further development of n‐type polymer conductivity. Herein, two alcohol‐soluble n‐type polythiophene derivatives that are n‐PT3 and n‐PT4 are reported. Due to the ability of two polymers to tolerate doping loading more significantly than 100 mol%, both achieve electrical conductivity >100 S cm−1. Moreover,...