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Bis(dimethylphenyl betaine) hydrochloride monohydrate was prepared and characterized by FTIR, Raman spectroscopes, and B3LYP/6-311++G(d,p) calculations. In the optimized structure of the complex, two betaine moieties are joined by a very strong asymmetric hydrogen bond with an O⋯O distance of 2.439Å. The water molecule is H-bonded to one oxygen atom of dimethylphenyl betaine and chloride anion via...
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