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The Raman spectra of CO2 molecules in hydrate cages was studied for structure I CO2 hydrate and structure II tetrahydrofuran (THF)+CO2 binary hydrate. The results obtained for sII hydrate indicated that the Fermi dyad peaks of CO2 in the small cage of THF–CO2 hydrate are located at 1274cm−1 and 1380cm−1. Numerical fitting of the sI CO2 hydrate Raman spectrum shows CO2 Fermi dyad peaks in the small...
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