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A semiclassical dynamics simulation study is reported for the ring opening reaction of 1,3-cyclohexadiene (CHD) triggered by a femtosecond-scale laser pulse. The results clearly demonstrate that, following the excitation by the laser pulse, the ring opening occurs at ∼110fs and the molecule decays to the ground electronic state at ∼210fs due to non-adiabatic transition of electrons from LUMO to HOMO...
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