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Stable cycling of LiCoO2 (LCO) cathode at high voltage is extremely challenging due to the notable structural instability in deeply delithiated states. Here, using the sol–gel coating method, LCO materials (LMP‐LCO) are obtained with bulk Mg‐doping and surface LiMgPO4/Li3PO4 (LMP/LPO) coating. The experimental results suggest that the simultaneous modification in the bulk and at the surface is demonstrated...
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