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A free-standing polypyrrole (PPy) film actuator without any additional electrode or metal backing, prepared electrochemically from an aromatic ester solution of tetra-n-butylammonium bis(trifluoromethanesulfonyl)imide (TBATFSI), exhibited up to 29% electrochemical strain, and a peak response rate of 10.8%s −1 in an H 2 O/propylene carbonate (PC) solution of LiTFSI. This is the very...
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