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Crystallographic, spectroscopic, and magnetic studies of three-center systems: lanthanoid-Ln3+ ions doubly-coordinated by TEMPO (2,2,6,6-tetramethylpiperidin-1-oxyl) radicals [Ln-TEMPO2] are reported. The temperature dependence of alternating-current magnetic susceptibility indicates the single-molecule-magnet behavior of Er-TEMPO2, exhibiting relatively slow magnetization relaxation. Well-resolved...
Spectroscopic and magnetic properties of uranium (5f 3 )- and lanthanide (4f N )-based single-ion magnets (SIMs) as well as single-molecule magnets (SMMs) are modelled using two interrelated crystal field (CF) approaches. The complete approach is based on the full Hamiltonian within the whole nf N configuration. This approach includes the free ion and CF terms, and thus it...
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