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We report an NMR study of electronic structure and wave functions overlap in the chain modification of semiconductor TlS which comprises two kinds of Tl atoms, Tl 1+ and Tl 3+ , residing in neighboring chains. Both univalent and trivalent Tl atoms show essential chemical shielding anisotropy despite of their 5d 10 6s 2 and 5d 10 electron...
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