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The chemical microenvironment modulation of metal nanoparticles (NPs) holds promise for tackling the long‐lasting challenge of the trade‐off effect between activity and selectivity in catalysis. Herein, ultrafine PdCu2 NPs incorporated into covalent organic frameworks (COFs) with diverse groups on their pore walls have been fabricated for the semihydrogenation of alkynes. The Cu species, as the primary...
The chemical microenvironment modulation of metal nanoparticles (NPs) holds promise for tackling the long‐lasting challenge of the trade‐off effect between activity and selectivity in catalysis. Herein, ultrafine PdCu2 NPs incorporated into covalent organic frameworks (COFs) with diverse groups on their pore walls have been fabricated for the semihydrogenation of alkynes. The Cu species, as the primary...
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