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Detailed molecular orbital and bonding analyses reveal the existence of both fluxional σ‐ and π‐bonds in the global minima Cs (1) and Cs MB18 (3) and transition states Cs (2) and Cs (4) of dianion and monoanions (M = K, Rb, and Cs). It is the fluxional bonds that facilitate the fluxional behaviors of the quasi‐planar and half‐sandwich which possess energy...
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