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The adsorption of CO and CO 2 on K-predosed Pd{110} at room temperature has been examined via reflection-absorption infrared spectroscopy (RAIRS). CO 2 adsorbs on 0.37 ML K-predosed Pd{110} with high sticking probability and a reactive chemisorbed intermediate, CO 2- , is detected in RAIRS at room temperature. Reaction of this species ultimately yields carbonate. The same...
Density functional theory calculations within the adiabatic coupling method have been performed for NO bound to Pd clusters exhibiting the structure appropriate to Pd{110} in order to estimate the influence of adsorption site on the NO stretching frequency. Three cluster sizes were investigated, with four, five and eight Pd atoms. In each case the NO bond length is found to be stretched, by 0.01 to...
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