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Tuning the coordination environment of the metal center in metal–nitrogen–carbon (M–N–C) single‐atom catalysts via heteroatom‐doping (oxygen, phosphorus, sulfur, etc.) is effective for promoting electrocatalytic CO2 reduction reaction (CO2RR). However, few studies are investigated establishing efficient CO2 reduction by introducing boron (B) atoms to regulate the M–N–C structure. Herein, a B‐C3N4...
Heteroatom‐doping is an effective method for modifying the geometric symmetry of metal–nitrogen–carbon (M–N–C) single‐atom catalysts and thereby tuning the electronic structure. Up to now, most of the current reports have concentrated on introducing heteroatoms into the highly symmetrical M–N4 structure. The coordination‐unsaturated M–N2 structure is more sterically favorable for the insertion of...
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