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Atmosphärenchemie J. S. Francisco, X. C. Zeng et al. zeigen in der Zuschrift auf S. 7848 ff., dass Criegee‐Intermediate mit hydrophoben Substituenten (länger als C1) länger auf der Oberfläche von Wassertröpfchen überleben.
Criegee intermediates have implications as key intermediates in atmospheric, organic, and enzymatic reactions. However, their chemistry in aqueous environments is relatively unexplored. Herein, Born–Oppenheimer molecular dynamics (BOMD) simulations examine the dynamic behavior of syn‐ and anti‐CH3CHOO at the air–water interface. They show that unlike the simplest Criegee intermediate (CH2OO), both...
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