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Caged to submission: The zinc‐ion‐directed assembly of tetrahedral protein cages (Zn30:CFMC‐112) in a rhombohedral crystal lattice is presented. The histidine side chains and exposed hydrophobic groups lining up the cavities of these cages enabled a flexible c‐type heme peptide fragment (a microperoxidase) to be immobilized within and its crystal structure to be determined at 1.9 Å resolution.
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