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The poor interface quality between nickel oxide (NiOx) and halide perovskites limits the performance and stability of NiOx‐based perovskite solar cells (PSCs). Here a reactive surface modification approach based on the in situ decomposition of urea on the NiOx surface is reported. The pyrolysis of urea can reduce the high‐valence state of nickel and replace the adsorbed hydroxyl group with isocyanate...
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