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The aminoacyl-β-ketophosphonate-adenosines (aa-KPA) are stable analogs of the aminoacyl adenylates, which are high-energy intermediates in the formation of aminoacyl-tRNA catalyzed by aminoacyl-tRNA synthetases (aaRS). We have synthesized glutamyl-β-ketophosphonate-adenosine (Glu-KPA) and glutaminyl-β-ketophosphonate-adenosine (Gln-KPA), and have tested them as inhibitors of their cognate aaRS, and...
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