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Ferroelectric photovoltaic (FPV) effect has been studied among a series of non‐stoichiometric BaTiO3 (Ba/Ti = 0.92–1.05) ceramic chips prepared by tape casting method. The FPV performance increases abruptly when the Ba/Ti molar ratio deviates from the stoichiometry within 1%. Meanwhile, a photocurrent direction switching behavior is observed between Ti‐excess and Ba‐excess samples. The TEM analysis...
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