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The development of novel building blocks with sp3‐hybridized‐carbon‐free conjugated skeletons is important to further advance and enrich nonfullerene acceptors (NFAs), but this remains a challenge due to the lack of strategies to effectively modulate the aggregation behavior of resulting NFAs. Herein, two novel nitrogen‐bridged octacyclic ladder‐type heteroarenes end‐capped with thiophene rings (BTPS)...
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