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The high overpotential in water oxidation on anodes is a limiting factor for the large‐scale application of photoelectrochemical cells. To overcome this limitation, it is essential to understand the four proton‐coupled electron transfer (PCET) steps in the reaction mechanism and their implications to the overpotential. Herein, a simple scheme to compute the energies of the PCET steps in water oxidation...
Protongekoppelter Elektronentransfer J. Cheng et al. nutzen in der Zuschrift auf S. 12242 ff. protonische Energieniveaus zur Beschreibung der Thermodynamik des protongekoppelten Elektronentransfers und veranschaulichen so die elektronischen und protonischen Beiträge zu thermodynamischen Überpotentialen in der Photokatalyse.
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