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Bio‐electrochemical conversion of anthropogenic CO2 into value‐added products using cost‐effective metal‐free catalysts represents a promising strategy for sustainable fuel production. Herein, N‐doped carbon nanosheets synthesized via pyrolysis of the zeolitic‐imidazolate framework (ZIF) are developed for constructing efficient biohybrids to facilitate CO2‐to‐CH4 conversion. The microbial enrichment...