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Tungsten‐based polyoxometalates (POMs) have been employed as UV‐driven photo‐catalysts for a range of organic transformations. Their photoactivity is dependent on electronic transitions between frontier orbitals and thus manipulation of orbital energy levels provides a promising means of extending their utility into the visible regime. Herein, an organic–inorganic hybrid polyoxometalate, K6[P2W17O...
Simple organic functionalization was shown to be a cost‐effective and durable approach to the visible‐light photoactivation of polyoxometalates (POMs). A new organic–inorganic hybrid polyoxometalate showed greatly enhanced photocatalytic activity in the visible region compared with analogous, non‐hybridized POM clusters. The new hybrid POM takes center stage in the cover art, illuminated by the sun...
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