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Methods to synthesize crystalline covalent triazine frameworks (CTFs) are limited and little attention has been paid to development of hydrophilic CTFs and photocatalytic overall water splitting. A route to synthesize crystalline and hydrophilic CTF‐HUST‐A1 with a benzylamine‐functionalized monomer is presented. The base reagent used plays an important role in the enhancement of crystallinity and...
Covalent triazine frameworks (CTFs) are normally synthesized by ionothermal methods. The harsh synthetic conditions and associated limited structural diversity do not benefit for further development and practical large‐scale synthesis of CTFs. Herein we report a new strategy to construct CTFs (CTF‐HUSTs) via a polycondensation approach, which allows the synthesis of CTFs under mild conditions from...
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