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An efficient polymer‐based catalytic system of poly(4‐vinylphenol) and tetra‐n‐butylammonium iodide was developed for the synthesis of cyclic carbonates from epoxides and CO2. Owing to the synergistic effects of hydroxyl groups and iodide anions, this commercially available and metal‐free system was highly active for the reaction of various terminal epoxides under environmentally benign conditions,...
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