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Two new metal‐free organic dyes, CR29 and CR52, with high extinction coefficients in the visible spectral region between 400–650 nm, have been synthesized. The donor–acceptor structure of the dyes feature benzodithiophene moieties BDT1 and BDT as rigid π‐conjugated spacers, which have so far been very little studied for dye‐sensitized solar cell (DSSC) applications. DFT/TDDFT calculations have been...
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