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It is a great challenge to simultaneously control the size, morphology, and facets of monodispersed Pd nanocrystals under a sub‐5 nm regime. Meanwhile, quantitative understanding of the thermodynamic and kinetic parameters to maneuver the shape evolution of nanocrystals in a one‐pot system still deserves investigation. Herein, a systematic study of the density functional theory (DFT)‐calculated adsorption...
In article number 1906026, Xiaoyu Qiu, Yawen Tang, and co‐workers systematically elucidate the explicit roles of adsorption energy, thermodynamic factors, and reduction kinetics on Pd growth patterns for achieving monodispersed sub‐5 nm Pd tetrahedrons and defect‐rich laciniate Pd nanourchins, which could serve as highly efficient non‐Pt catalysts for both the oxygen reduction reaction and the formic...
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