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The role of band structure in heterogeneous electron transfer kinetics at graphene and carbon nanotube electrodes is discussed within Gerischer‐Marcus model. Raman spectroscopy was used to estimate the averaged density of defects in anodized epitaxial graphene, single‐walled carbon nanotube mats, and multi‐walled carbon nanotube carpets. Comparison of the density of defects with cyclic voltammetry...
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