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Anionenkoordination an einen verbrückten Hafnocen‐Nitrid‐Komplex, der durch CO‐induzierte N2‐Spaltung erhalten wurde, erhöht die Nucleophilie des N‐Atoms und fördert so eine zusätzliche N‐C‐Bindungsbildung mit einem typischerweise inerten terminalen Isocyanatliganden. Diese Kaskadensequenz ermöglicht die Synthese von sonst schwer zugänglichen, monosubstituierten Harnstoffen mithilfe von N2, CO und...
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