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Cooperative interaction between multiple chiral centers dictates the absolute handedness of structural folding. We have designed and prepared a series of chiral C3‐symmetric tris(N‐salicylidenamine) derivatives that adopt three‐blade propeller‐like conformations. Synthetic access to an expanded family of such constructs was aided by enzymatic resolution and C–C cross‐coupling reactions of aryl‐substituted...
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