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To make full use of the renewability of polylactide (PLA) and natural Eucommia ulmoides gum (EUG), novel fully sustainable thermal plastic vulcanizates (TPVs) with high toughness were developed via dynamic vulcanization technique based on modified EUG (referred to as EUG‐GMA). The latter greatly improved the toughness of PLA and the mechanism was discussed with respect to micro structure analysis...
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