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Based on the chiral helicene‐derived dipyridyl ligands, two pairs of chiral rhomboid metallacycles were constructed conveniently by the coordination‐driven self‐assembly. It was found that the chiral metallacycles showed a supramolecular depiction of the illusory Penrose stairs. Moreover, the enantiomers of the metallacycles not only showed clear mirror imaged circular dichroism (CD) spectra and mirror...
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