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We demonstrate that the imidazole‐based ligand 1 efficiently produces a coordination polymer gel by simple mixing with Co2+ ion. When the molar ratio of CoCl2 to ligand 1 was less < 1, a red sol was obtained, indicating the formation of an octahedral (Oh) complex species as occurs with Co(NO3)2. In contrast to G1, when the amount of CoCl2 employed was more than 1 equiv., the color of the gel changed...
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