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The two ligands 2,6‐bis(4‐methylquinolin‐2‐yl)pyridine (L1) and diethyl 2,2′‐(pyridine‐2,6‐diyl)bis(quinolone‐4‐carboxylate) (L2) were used to prepare the homoleptic [Ru(L2)2][PF6]2 (RU1) and heteroleptic [Ru(L1)(L2)][PF6]2 (RU2) complexes. DFT calculations (B3PW91,3‐21G**) performed on both RU1 and RU2 revealed that redox at the ruthenium site for RU2 is less positive by ca. 110 mV. Consequently,...
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