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Polymer solar cells (PSCs) rely on a blend of small molecular acceptors (SMAs) with polymer donors, where thermodynamic relaxation of SMAs poses critical concerns on operational stability. To tackle this issue, tethered SMAs, wherein multiple SMA‐subunits are connected to the aromatic‐core via flexible chains, are proposed. This design aims to an elevated glass transition temperature (Tg) for a dynamical...
Polymer solar cells (PSCs) rely on a blend of small molecular acceptors (SMAs) with polymer donors, where thermodynamic relaxation of SMAs poses critical concerns on operational stability. To tackle this issue, tethered SMAs, wherein multiple SMA‐subunits are connected to the aromatic‐core via flexible chains, are proposed. This design aims to an elevated glass transition temperature (Tg) for a dynamical...