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The binding positions (terraces, steps) and sites (on-top, bridge-bonded, threefold) of adsorbed CO have been studied on Pd(S)-[n(111)×(111)] (n=2, 3, 5, 9, 20, ∞) and Pd(S)-[n(100)×(111)] (n=2, 5, 9, ∞) electrodes in 0.1M HClO 4 saturated with CO using infrared reflection absorption spectroscopy (IRAS). The band of threefold CO is observed around 1950cm −1 on Pd(S)-[n(111)×(111)]...
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