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Biomimetic cross‐linked polymersomes that exhibit a self‐beating motion without any on–off switching are developed. The polymersomes are made from a well‐defined synthetic thermoresponsive diblock copolymer, and the thermoresponsive segment includes ruthenium catalysts for the oscillatory chemical reaction and vinylidene groups to cross‐link the polymersomes. Autonomous volume and shape oscillations...
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