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To realize a renewable energy society, a polymeric system for photoinduced hydrogen generation utilizing a copolymer containing an electron acceptor was designed. In this system, the redox changes of viologen introduced into poly(N‐isopropylacrylamide) cause cyclic conformational changes owing to the shifting of the phase transition temperature (PTT). The polymeric coil–globule transitions with hydrophilic/hydrophobic...
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