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The [3 + 2] cycloaddition (32CA) reaction of benzonitrile oxide, BNO 2, with an electron‐rich N‐vinylpyrrole derivative, NVP 3a, in the presence of dichloromethane, has been theoretically studied using density functional theory (DFT) methods at the B3LYP/6‐31G(d) level. This 32CA reaction presents a relatively high activation Gibbs free energy as a result of the low polar character of this zwitterionic‐type...
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