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Treatment of [2‐(2‐bromophenyl)allyl]trimethylsilane with tBuLi in THF at –78 °C resulted in the rapid migration of the trimethylsilyl group to afford an allylic organolithium that can be easily trapped by a wide range of electrophiles. This is a rare example of a synthetically useful and efficientcarbon‐to‐carbon migration of a silicon group and represents a new approach to allylic organolithium...
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