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Amongst various Fenton‐like single‐atom catalysts (SACs), the zinc (Zn)‐related SACs have been barely reported due to the fully occupied 3d10 configuration of Zn2+ being inactive for the Fenton‐like reaction. Herein, the inert element Zn is turned into an active single‐atom catalyst (SA−Zn−NC) for Fenton‐like chemistry by forming an atomic Zn−N4 coordination structure. The SA−Zn−NC shows admirable...