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Synergic combinations of alkali‐metal hydrocarbyl/amide reagents were used to synthesise saturated N‐heterocyclic carbene (NHC) ligands tethered to a fluorenide anion through deprotonation of a spirocyclic precursor, whereas conventional bases were not successful. The Li2 derivatives displayed a bridging amide between two Li atoms within the fluorenide‐NHC pocket, whereas the Na2 and K2 analogues...
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