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Unprecedented intense fluorescent emission was observed for a variety of flavin compounds bearing a perpendicular cyclic imide moiety at the C7 position of an isoalloxazine platform. A series of alloxan‐substituted flavins was prepared selectively by reduction of the corresponding N‐aryl‐2‐nitro‐5‐alkoxyanilines with zinc dust and subsequent reaction with alloxan monohydrate in the presence of boric...
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