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Photothermal CO2 hydrogenation to high‐value‐added chemicals and fuels is an appealing approach to alleviate energy and environmental concerns. However, it still relies on the development of earth‐abundant, efficient, and durable catalysts. Here, the design of N‐doped carbon‐coated Co nanoparticles (NPs), as a photothermal catalyst, synthesized through a two‐step pyrolysis of Co‐based ZIF‐67 precursor,...