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Anders als bisher angenommen, ist die Bildung eines kationischen hydratisierten Titan(III)‐Komplexes essenziell für die Aktivierung von H2O für Wasserstoffatom‐Transferreaktionen. Die relevanten Intermediate wurden über moderne EPR‐Methoden (siehe Spektrum) und Cyclovoltammetrie charakterisiert. Die Strukturzuordnungen wurden durch theoretische Rechnungen bestätigt, und berechnete BDEs sind nun in...
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