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Reactions of a trivalent diboryl Ir complex Ir-(Bpin)2 supported with a POCOP-type pincer ligand with a series of small molecules have been explored (pin = pinacolate). Ir-(Bpin)2 deoxygenated CO2 to make Ir-CO and O(Bpin)2. Attempts to deoxygenate other carbonyl compounds were not successful. The reaction with CO led to loss of B2pin2 by reductive elimination and its replacement on Ir with CO. Ir-(Bpin)...
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