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Compressive chiral hydrogels are fabricated from thermoresponsive helical dendronized poly(phenylacetylene)s through dynamic covalent chemistry at freezing temperature. These highly porous hydrogels possess stabilized chiralities originated from the copolymer precursors, and exhibit remarkable compressibility like human articular cartilage with full recoverability and excellent fatigue resistance,...
Der Phasenübergang von thermoresponsiven dendronisierten Polymeren wurde durch CW‐EPR‐Spektroskopie auf molekularer Ebene charakterisiert. Die Aggregation des Polymers wird durch dynamische, nanometergroße Strukturinhomogenitäten eingeleitet, und die Dehydratisierung der Polymerketten zieht sich trotz des makroskopisch scharfen Phasenübergangs über einen Temperaturbereich von mindestens 30 K hin (siehe...
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